Saccharin: a cheap and mild acidic agent for the synthesis of azo dyes via telescoped dediazotization

Document Type

Article

Publication Date

1-1-2019

Abstract

Green synthesis methods are considered as a safer alternative to the conventional synthetic processes due to their eco-friendly nature, cost-effectiveness, and easy handling. In the present study, an eco-friendly and sustainable method for the synthesis of stable arenediazonium has been developed using saccharin as a cheap and mild acidic agent and tert-butyl nitrite as a diazotization reagent for the first time. These stable intermediates were used in the azo coupling reaction with 4-hydroxybenzaldehyde via telescoped dediazotization. The current method has advantages such as reduced waste by avoiding solvent for the purification of intermediate in diazotization step, cost-effectiveness, simple experimental procedure, good yield of azo dyes, metal-free waste, and environmentally benign conditions. An interesting aspect of this study is the recovery of saccharin from the reaction, which could be reused. © 2019 Walter de Gruyter GmbH, Berlin/Boston.

Keywords

azo coupling, cost-effectiveness, saccharin, stable arenediazonium, sustainable protocol

Divisions

nanotechnology

Funders

High Impact Research Grant (no. RP025A/B/C-14AET) for Scientific Research from University of Malaya, Malaysia

Publication Title

Green Processing and Synthesis

Volume

8

Issue

1

Publisher

De Gruyter

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