1,1′-Butylenebis(3-sulfo-3H-imidazol-1-ium) hydrogensulfate: a versatile task-specific ionic liquid catalyst for the synthesis of 4H-pyran scaffolds through non-conventional process

Document Type

Article

Publication Date

1-1-2019

Abstract

Abstract: In the present study, the catalytic efficiency of 1,1′-butylenebis(3-sulfo-3H-imidazol-1-ium) hydrogensulfate (BBSI-HSO 4 ) as a versatile sulfonic acid-functionalized ionic liquid was demonstrated for the one-pot mechanosynthesis of pyrano[4,3-b]-pyrans using planetary ball mill at room temperature under solvent-free conditions. This efficient mechanosynthesis approach to the 4H-pyran scaffolds displays a combination of the structure–activity relationship of ionic liquids with ecological benefits of a mechanocatalytic procedure. The ionic liquid was easily recycled and reused several times with no significant loss of its catalytic activity. Graphical abstract: [Figure not available: see fulltext.]. © 2019, Springer-Verlag GmbH Austria, part of Springer Nature.

Keywords

4H-Pyran, Ball milling process, Mild conditions, Recyclable catalyst, Structure–activity relationship, Sulfonic acid-functionalized ionic liquid

Divisions

nanotechnology

Publication Title

Monatshefte fur Chemie - Chemical Monthly

Volume

150

Issue

4

Publisher

Springer Verlag

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