Detecting adulteration of stingless bee honey using untargeted H-1 NMR metabolomics with chemometrics

Document Type

Article

Publication Date

1-30-2022

Abstract

As stingless bee honey (SBH) is gaining in popularity in the Malaysian market, it is now prone to adulteration. The higher price of SBH compared to floral honey has led to the use of unusual adulterants such as vinegar and even floral honey to mimic the unique taste and appearance of SBH. Since the current AOAC 998.12 method fails to detect these adulterants as their delta C-13 values are in the range for C-3 plants, untargeted H-1 NMR metabolomics was proposed. Principal component analysis of SBH H-1 NMR fingerprints was able to distinguish authentic SBHs from adulterated ones down to 1% adulteration level for selected adulterants. Discriminant analysis showed promising results in distinguishing the preliminary datasets of authentic SBHs from the adulterated ones, including discriminating SBHs adulterated with different adulterants derived from C-3 and C-4 plants. Hence, to assure any emerging adulterant can be detected, all H-1 NMR regions should be considered.

Keywords

Chemometrics, Honey adulteration, Metabolomics, NMR, Stingless bee honey

Divisions

pharmacy

Funders

Ministry of Higher Education, Malaysia under the Fundamental Research Grant Scheme (FRGS) [Grant No: USM 203/PTEKIND/6711612],Kuok Foundation

Publication Title

Food Chemistry

Volume

368

Publisher

Elsevier Science Ltd

Publisher Location

THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND

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