Characteristics of plasticized lithium ion conducting green polymer blend electrolytes based on cs: Dextran with high energy density and specific capacitance

Document Type

Article

Publication Date

11-1-2021

Abstract

The solution cast process is used to set up chitosan: dextran-based plasticized solid polymer electrolyte with high specific capacitance (228.62 F/g) at the 1st cycle. Fourier-transform infrared spectroscopy (FTIR) pattern revealed the interaction between polymers and electrolyte components. At ambient temperature, the highest conductive plasticized system (CDLG-3) achieves a maximum conductivity of 4.16 x 10(-4) S cm(-1). Using both FTIR and electrical impedance spectroscopy (EIS) methods, the mobility, number density, and diffusion coefficient of ions are measured, and they are found to rise as the amount of glycerol increases. Ions are the primary charge carriers, according to transference number measurement (TNM). According to linear sweep voltammetry (LSV), the CDLG-3 system's electrochemical stability window is 2.2 V. In the preparation of electrical double layer capacitor devices, the CDLG-3 system was used. There are no Faradaic peaks on the cyclic voltammetry (CV) curve, which is virtually rectangular. Beyond the 20th cycle, the power density, energy density, and specific capacitance values from the galvanostatic charge-discharge are practically constant at 480 W/Kg, 8 Wh/Kg, and 60 F g(-1), for 180 cycles.

Keywords

Solid polymer electrolyte, Impedance, Transport properties, FTIR study, Electrochemical double-layer capacitor device

Divisions

foundation

Funders

University of Sulaimani,Komar University of Science and Technology,Taif University, Taif, Saudi Arabia [Grant No: TURSP-2020/162],Prince Sultan University

Publication Title

Polymers

Volume

13

Issue

21

Publisher

MDPI

Publisher Location

ST ALBAN-ANLAGE 66, CH-4052 BASEL, SWITZERLAND

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