In-depth thermal, microstructural and photoluminescence analysis of mesoporous ZnO/ZnAl2o4-MMO: The effect of molar ratio

Document Type

Article

Publication Date

10-1-2021

Abstract

This manuscript reports a detailed preparation and characterization of mesoporous ZnO/ZnAl2O4 mixed metal oxide (MMO) through a two-step solution procedure utilizing Zn/Al layered double hydroxide (LDH) as starting materials. The influence of the molar ratio was comprehensively explored via a number of characterization techniques. Field emission scanning electron microscopy analysis revealed the occurrence of a sheet-like morphology with thickness of 65 nm at molar ratio (r = 6). Simultaneously, a mesoporous nature of the deposited film was observed through the surface area analysis. A considerable value of surface area was obtained (53.3 m(2) g(-1)) through which a high amount of dye was loaded on the deposited film (3.3 x 10(-4)); the latter was evaluated via a regression equation in conjunction with the ultraviolet visible light analysis. This in turn led to a robust correlation between the anticipated surface area, pore size, and the estimated dye loading amount. Moreover, the optical and photoluminescence (PL) features were investigated using UV-vis and PL techniques, wherein the near-band emission (was observed at around 380 nm. The proposed work may provide an alternative eco-friendly approach for future visible light photodetector application.

Keywords

Mesoporous ZnO/ZnAl2O4, Mixed metal oxide (MMO), Photodetector application, Ultraviolet visible light analysis, Layered double hydroxide

Divisions

fac_eng

Funders

Deputyship for Research & Innovation, Ministry of Education in Saudi Arabia [Grant no: 375213500],Central laboratory at Jouf University,King Khalid University

Publication Title

ECS Journal of Solid State Science and Technology

Volume

10

Issue

10

Publisher

Electrochemical Soc Inc

Publisher Location

65 SOUTH MAIN STREET, PENNINGTON, NJ 08534 USA

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