Impact of reactor materials on methane decomposition for hydrogen production

Document Type

Article

Publication Date

10-1-2021

Abstract

In this study, the catalytic effect of the internal surface of reactors constructed from stainless steel (SS310) for hydrogen production via methane decomposition has experimentally been proved and compared with a quartz-lined reactor. The effects of the methane decomposition temperature and volume-hourly-space velocity (VHSV) on hydrogen production, conversion of methane, and initial decomposition rates were investigated in an SS310 lab-scale reactor. Within the duration of the experiments, no change was recorded for hydrogen and methane concentration in all the experiments. The catalytic activity of the SS310 reactor's internal surface increased with increasing methane decomposition temperature (850-950 degrees C) and decreasing VHSV (37-52 h(-1)). The as-produced carbon was characterized using surface texture analysis, X-ray, and SEM-EDX. (C) 2021 Published by Elsevier B.V. on behalf of Institution of Chemical Engineers.

Keywords

Catalytic methane decomposition, Hydrogen production, Activated carbon, Reactor effect

Divisions

sch_che

Publication Title

Chemical Engineering Research & Design

Volume

174

Publisher

Elsevier

Publisher Location

RADARWEG 29, 1043 NX AMSTERDAM, NETHERLANDS

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