Iron oxide nanoparticles decorated oleic acid for high colloidal stability

Document Type

Article

Publication Date

1-1-2017

Abstract

In the present study, oleic acid (OA)-decorated magnetite nanoparticles (MNPs) were synthesized via in situ co-precipitation method using ammonium hydroxide as a precipitating agent. This study aims to determine the optimum loading amount of OA for improving the MNPs colloidal stability. Based on our results obtained, it was found that the zeta potential values of MNPs increased from −29.8 to −58.1 mV after modification of MNPs with 1.2 wt.% of OA. Indeed, results obtained clearly to show that a maximum colloidal stability of MNPs in a basic medium could be significantly improved. As a result, this resultant colloidal suspension performance was approximately 7 times higher (21 days- high colloidal stability against precipitation and agglomeration) than that of the undecorated MNPs sample (3 days). Based on vibrating sample magnetometer (VSM) analysis, the resultant OA-decorated MNPs exhibited superparamagnetic behavior with slightly lower saturation magnetization (51–69 emu/g) than that of undecorated MNPs sample (80 emu/g) at room temperature. This behavior was attributed to the sufficient carboxylate ions from the outer layer of the bilayer of OA-decorated MNPs, which promoted the high colloidal stability performance.

Keywords

colloidal stabsility, magnetite nanoparticles, oleic acid, superparamagnetic

Divisions

nanotechnology

Funders

University of Malaya: Fundamental Research Grant Scheme (FP008-2015A), Grand Challenge Grant (GC002A-15SBS), University Malaya Research Fund Assistance (BK096-2016), and University of Malaya Postgraduate Research Grant (PG068-2014B) and PG061-2014B

Publication Title

Advances in Polymer Technology

Volume

37

Issue

6

Publisher

Wiley

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