Basophilic method for lanthanide MOFs with a drug ligand: Crystal structure and luminescence

Document Type

Article

Publication Date

1-1-2015

Abstract

Recently developed basophilic method was adopted to synthesize phenolic hydroxyl bridged lanthanide MOFs (Ln-MOFs) 1 and 2, based on a drug ligand of salicylic acid. 1 and 2 have the general formula of [Ln(HL1)L1·H2O]n (H2L1 = salicylic acid, Ln = Tb and Gd), they are characterized by X-ray single crystal diffraction, fourier transform infrared (FT-IR), elemental analysis (EA), thermogravimetric analysis (TGA) and powder X-ray diffraction (PXRD). It is found that the Ln Ln distance will be shorter if more phenolic hydroxyl as bridges, this will lead to more rigid framework and suggesting that the hydroxyl bridged CPs are good candidates for photophysical and magnetic materials. Furthermore, the luminescence property of 1 was investigated.

Keywords

Basophilic method, Lanthanide MOFs, Drug ligand, Crystal structure, Luminescence

Divisions

CHEMISTRY

Funders

Jiangxi Normal University (5616),University of Malaya (UM.C/625/1/HIR/247)

Publication Title

Inorganica Chimica Acta

Volume

432

Publisher

Elsevier

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